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I like this song for the series since its lyrics are about travelling, exploring and seeking.
Around the World - Monkey Majik
for the end of the chimera ant arc ending
(where meurem and komugi die)
w-inds be as one
The guy who used Stratovarius' Hunting High and Low and the guy who mentioned Ten Masked Men's You Spin Me Round cover nailed it.
For Illumi I think Castlevania Symphony of the Night's Door to the Abyss fits him well.
Hisoka: Possibly Municipal Waste's Sadistic Magician.
There's this one that reminded me of the themes of friendship and adventure in the story: http://www.youtube.com/watch?v=TeiikKQQ3Dk
Then there's this one, just before the palace assault, it starts of slowly when each one in the group is concentrating on what he's gonna do next, then it gets off when it's time and they enter the palace from Nov's gate: http://www.youtube.com/watch?v=HTgdeM4XoBU
Ging being epic and travelling the world on his dragons' back: http://www.youtube.com/watch?v=2hClyvvZh3w
Kakin's emperor's announcement and Beyond's speech: http://www.youtube.com/watch?v=enlTFVgWN1g
Netero's fight: http://www.youtube.com/watch?v=xjKdGSkuSFA
Ok maybe I went a bit overboard, but still I think it's awesome music!